The transport properties of an artificial single-molecule magnet based on a CdTe quantum dot doped with a single Mn＋2 ion（S=5/2） are investigated by the non-equilibrium Green function method.We consider a minimal model where the Mn-hole exchange coupling is strongly anisotropic so that spin-flip is suppressed and the impurity spin S and a hole spin s entering the quantum dot are coupled into spin pair states with（2S＋1） sublevels.In the sequential tunneling regime,the differential conductance exhibits（2S＋1） possible peaks,corresponding to resonance tunneling via（2S＋1） sublevels.At low temperature,Kondo physics dominates transport and（2S＋1） Kondo peaks occur in the local density of states and conductance.These peaks originate from the spin-singlet state formed by the holes in the leads and on the dot via higher-order processes and are related to the parallel and antiparallel spin pair states.
We study the thermoelectric transport through a double-quantum-dot system with spin-dependent interdot cou- pling and ferromagnetic electrodes by means of the non-equilibrium Green＇s function in the linear response regime. It is found that the thermoelectric coefficients are strongly dependent on the splitting of the interdot coupling, the relative magnetic configurations, and the spin polarization of leads. In particular, the thermoelectric efficiency can reach a considerable value in the parallel configuration when the effective interdot coupling and the tunnel coupling between the quantum dots and the leads for the spin-down electrons are small. Moreover, the thermoelectric efficiency increases with the intradot Coulomb interaction increasing and can reach very high values at appropriate temperatures. In the presence of the magnetic field, the spin accumulation in the leads strongly suppresses the thermoelectric efficiency, and a pure spin thermopower can be obtained.
